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Movie version of the Shinsengumi Crisis arc (episodes 101-105) and the Kabukicho Four Devas arc (episodes 210-214) which were screened in selected theaters in Japan.
AnimeLok is the best site to watch Gintama: Yorinuki Gintama-san on Theater 2D SUB online, or you can even watch Gintama: Yorinuki Gintama-san on Theater 2D DUB in HD quality. You can also find Sunrise anime on AnimeLok website.
